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rdf:type
lifeskim:mentions
pubmed:issue
16
pubmed:dateCreated
2011-4-7
pubmed:abstractText
In the pyrochlore Yb(2)GaSbO(7), the Yb(3+) sublattice forms a network of corner sharing tetrahedra and the second sublattice is made up of disordered, non-magnetic Ga(3+) and Sb(5+) ions. We have examined this compound using magnetic susceptibility, (170)Yb Mössbauer spectroscopy (down to 0.03 K) and muon spin relaxation (?SR) (down to 0.02 K) measurements. We establish the size of the Yb(3+) magnetic moments and that of the Yb(3+)-Yb(3+) coupling. At low temperatures, the correlated moments fluctuate between directions that are well tilted relative to the local [111] axis. The lattice disorder does not quench the frustration induced low temperature spin fluctuations but it does remove the first order dynamic transition that is present in the crystallographically ordered counterpart Yb(2)Ti(2)O(7). Below 1.0 K, the fluctuation rate of the correlated moments decreases progressively as the temperature is reduced and the moments remain dynamic down to 0.02?K where the rate is 7 × 10(7) s(-1). Magnetic frustration is operative in Yb(2)GaSbO(7) where the Yb(3+)-Yb(3+) interaction is antiferromagnetic as it is in Yb(2)Ti(2)O(7) where the interaction is ferromagnetic.
pubmed:language
eng
pubmed:journal
pubmed:status
PubMed-not-MEDLINE
pubmed:month
Apr
pubmed:issn
1361-648X
pubmed:author
pubmed:issnType
Electronic
pubmed:day
27
pubmed:volume
23
pubmed:owner
NLM
pubmed:authorsComplete
Y
pubmed:pagination
164217
pubmed:year
2011
pubmed:articleTitle
Magnetic frustration in the disordered pyrochlore Yb(2)GaSbO(7).
pubmed:affiliation
CEA-Saclay, IRAMIS/SPEC, F-91191 Gif sur Yvette, France.
pubmed:publicationType
Journal Article