Linked Life Data

19577276

Source:http://linkedlifedata.com/resource/pubmed/id/19577276

Statements in which the resource exists as a subject.
PredicateObject
rdf:type
lifeskim:mentions
pubmed:issue
9
pubmed:dateCreated
2009-8-11
pubmed:abstractText
The influence of multicomponent additives on NO reduction by selective non-catalytic reduction process has been investigated experimentally in an electricity-heated tube reactor. The multicomponent additives are composed of two species of CO, CH(4) and H(2), and the molar ratio of their two components varies from 1/3 to 3/1. The results show that all the investigated additives could decrease the optimal temperature for NO reduction effectively, but the contributions of their components are different. The performance of multicomponent additive composed of CO and CH(4) depends mainly on CH(4) component. The function of CO component is shifting the temperature window for NO reduction to lower temperature slightly and narrowing the temperature window a little. The temperature window with multicomponent additive composed of H(2) and CH(4) is distinct from that with its each component, so both H(2) and CH(4) component make important contributions. While the fraction of CO is no more than that of H(2) in multicomponent additives composed of them, the performance of multicomponent additives is dominated by H(2) component; while the fraction of CO becomes larger, the influence of CO component becomes notable. Qualitatively the modeling results using a detailed chemical kinetic mechanism exhibit the same characteristics of the temperature window shift as observed experimentally. By reaction mechanism analysis, the distinct influences of CO, CH(4) or H(2) component on the property of multicomponent additive are mainly caused by the different production rates of (*)OH radical in their own oxidation process.
pubmed:language
eng
pubmed:journal
pubmed:citationSubset
IM
pubmed:chemical
pubmed:status
MEDLINE
pubmed:month
Aug
pubmed:issn
1879-1298
pubmed:author
pubmed:issnType
Electronic
pubmed:volume
76
pubmed:owner
NLM
pubmed:authorsComplete
Y
pubmed:pagination
1199-205
pubmed:meshHeading
pubmed:year
2009
pubmed:articleTitle
Experimental and modeling study of the effects of multicomponent gas additives on selective non-catalytic reduction process.
pubmed:affiliation
School of Energy Science and Engineering, Harbin Institute of Technology, Harbin 150001, PR China. caoqx@hit.edu.cn
pubmed:publicationType
Journal Article, Research Support, Non-U.S. Gov't