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rdf:type
lifeskim:mentions
pubmed:issue
9
pubmed:dateCreated
2006-4-11
pubmed:abstractText
We analyze distributions of exciton populations in PbSe nanocrystal (NC) ensembles as a function of excitation wavelength. For photon energies that result in carrier multiplication, these distributions are non-Poissonian and are characterized by two dominant exciton multiplicities that are determined by the ratio of photon energy to NC energy gap. For certain photon energies, we produce photoexcited NC ensembles with a nearly pure single multiplicity that can be tuned from 1 to 7. This result can find applications ranging from lasing and nonlinear optics to photovoltaics and photocatalysis.
pubmed:language
eng
pubmed:journal
pubmed:status
PubMed-not-MEDLINE
pubmed:month
Mar
pubmed:issn
0031-9007
pubmed:author
pubmed:issnType
Print
pubmed:day
10
pubmed:volume
96
pubmed:owner
NLM
pubmed:authorsComplete
Y
pubmed:pagination
097402
pubmed:year
2006
pubmed:articleTitle
Non-Poissonian exciton populations in semiconductor nanocrystals via carrier multiplication.
pubmed:affiliation
Chemistry Division, C-PCS, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA.
pubmed:publicationType
Journal Article