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PredicateObject
rdf:type
lifeskim:mentions
pubmed:issue
17
pubmed:dateCreated
2004-11-4
pubmed:abstractText
A quantitative determination of 2s vacancy lifetimes in surface and bulk atoms of free Ne clusters has been made. While for free atoms the 2s inner-valence hole has a ps lifetime, it reduces to 6+/-1 fs for cluster bulk atoms. For surface atoms, the lifetime is on average longer than 30 fs. The lifetime estimate was obtained from fits of high-resolution photoelectron spectra of Ne clusters. The shortening of the lifetime is attributed to the coordination dependent interatomic Coulombic decay, which is extremely sensitive to internuclear distances.
pubmed:language
eng
pubmed:journal
pubmed:status
PubMed-not-MEDLINE
pubmed:month
Oct
pubmed:issn
0031-9007
pubmed:author
pubmed:issnType
Print
pubmed:day
22
pubmed:volume
93
pubmed:owner
NLM
pubmed:authorsComplete
Y
pubmed:pagination
173401
pubmed:year
2004
pubmed:articleTitle
Femtosecond interatomic Coulombic decay in free neon clusters: large lifetime differences between surface and bulk.
pubmed:affiliation
Department of Physics, Uppsala University, Box 530, S-751 21 Uppsala, Sweden. gunnar.ohrwall@fysik.uu.se
pubmed:publicationType
Journal Article