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pubmed-article:16968043pubmed:abstractTextHigh-resolution spectral hole-burning studies of CdSe/ZnS core/shell nanorods reveal a sharp zero-phonon line, with a line width dependent on the measurement time scale. The zero-phonon line width is attributed to contributions from radiative decay, spectral diffusion induced by surface electric field fluctuations, and phonon-assisted migration of excitons localized in the nanorods. A decoherence rate as small as 4.5 GHz has been observed, when the effects of spectral diffusion are suppressed in the spectral hole-burning measurement. Comparison between zero-phonon line widths in nanorods and spherical nanocrystals also elucidates important differences in the decoherence process between the one- and zero-dimensional nanostructures.lld:pubmed
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pubmed-article:16968043pubmed:authorpubmed-author:WangHailinHlld:pubmed
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pubmed-article:16968043pubmed:dateRevised2006-11-15lld:pubmed
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pubmed-article:16968043pubmed:year2006lld:pubmed
pubmed-article:16968043pubmed:articleTitleZero-phonon linewidth in CdSe/ZnS core/shell nanorods.lld:pubmed
pubmed-article:16968043pubmed:affiliationDepartment of Physics, University of Oregon, Eugene, Oregon 97403, USA.lld:pubmed
pubmed-article:16968043pubmed:publicationTypeJournal Articlelld:pubmed
pubmed-article:16968043pubmed:publicationTypeResearch Support, U.S. Gov't, Non-P.H.S.lld:pubmed